Stretchable and ultraflexible electronic devices have a broad range of potential uses, from robust devices for energy storage and conversion to biomedical devices that make conformal interfaces with the skin and internal organs. Organics have long been associated with mechanical compliance, which enables inexpensive manufacturing via roll-to-roll printing. This article provides an overview of the use of organic electronic materials, including π-conjugated polymers and small molecules, in highly deformable devices. It begins with a comparison of devices based on organic devices to those based on inorganic composites. The thin-film nature of organic semiconductor devices has also led to the development of several techniques for metrology that can be applied specifically to brittle organic thin films. The article concludes with a brief discussion of the applications of stretchable and ultraflexible organic electronic devices and a prescriptive outlook for successful collaborative work in this exciting, interdisciplinary field.
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